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CO2 has been addressed as a greenhouse gas in recent years. Thus, CO2 is included in the greenhouse gas inventory of the Kyoto Protocol and was also considered in the United Nations Framework Convention on Climate Change (UNFCCC). However, CO2-based technologies are still in infancy. In this paper, we review recent research efforts in CO2 sorption on oxide materials. First, we discuss the CO2 sorption on metal oxides, including recent experimental and theoretical investigations, using three types of computational approaches: density functional theory (DFT), the random phase approximation (RPA), and the super cell method. Then, an overview of CO2 sorption on oxide materials, including metal oxides and metal-doped oxides, which are used for CO2 capture and carbon capture and sequestration (CCS) is provided. Finally, on the basis of the recent results, comprehensive understandings of CO2 adsorption on oxide materials and the corresponding practical applications are suggested. In this paper, CO2 sorption is addressed in terms of gas-solid interaction, CO2 adsorption, gas-solid charge transfer, surface reaction, and surface reaction kinetics. For each type of gas-solid interaction, the effect of gas-phase CO2 concentration, surface coordination, and surface defect on CO2 adsorption is summarized. Also, the adsorption mechanism of CO2 on metal oxides is discussed. Finally, the reasons for low CO2 adsorption on oxide materials are analyzed with respect to the gas-solid interactions, CO2 adsorption, and surface reactions. The results in this review highlight the possibility of CO2 capture and CCS, which could be, however, limited by surface reaction and the corresponding reaction kinetics. Achieving a balance between CO2 capture and surface reaction is therefore suggested.

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